Coming from a WSDL Contract Perspective, each operation can can have at most one response. However, you can define multiple fault contracts, which basically tells a client "Expect either a response defined by DataContractX or a fault response defined by FaultContractY or FaultContractZ .
It can depend on where and how you want the exception handled. A client (regardless of platform) will always receive a soap fault exception whether the service code doesn't catch the exception or the service throws a FaultException or the generic version.
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